This collaborative project between the University of Maryland, Baltimore County (UMBC) and the University of Illinois Urbana-Champaign (UIUC) addresses the research and educational aspects of combining AI and Cybersecurity. Our goals are to (1) carry out novel research on applying the latest AI techniques to cybersecurity problems and explore how attacks on AI systems can be mitigated, (2) extend our innovative work on evaluating students understanding of the underlying security concepts to include AI-related topics, and (3) create and evaluate modules and exercises for undergraduate, graduate and professional courses on both cybersecurity and AI to cover the concepts, examples, and tools illustrating how they can support one another.